Thickness dependence of dynamic and static magnetic properties of pulsed laser deposited La0.7Sr0.3MnO3 films on SrTiO3(001)

Åsmund Monsen, Jos E. Boschker, Ferran Macià, Justin W. Wells, Per Nordblad, Andrew D. Kent, Roland Mathieu, Thomas Tybell, Erik Wahlström

    Research output: Contribution to journalArticle

    Abstract

    We present a comprehensive study of the thickness dependence of static and magneto-dynamic magnetic properties of La0.7Sr0.3MnO 3. Epitaxial pulsed laser deposited La0.7Sr 0.3MnO3/SrTiO3(001) thin films in the range from 3 unit cell (uc) to 40 uc (1.2-16 nm) have been investigated through ferromagnetic resonance (FMR) spectroscopy and SQUID magnetometry at variable temperature. Magnetodynamically, three different thickness, d, regimes are identified: 20 uc ≲d uc where the system is bulk like, a transition region 8 uc ≤≲20 uc where the FMR linewidth and the position depend on thickness and d=6 uc which displays significantly altered magnetodynamic properties, while still displaying bulk magnetization. Magnetization and FMR measurements are consistent with a nonmagnetic volume corresponding to ∼4 uc. We observe a reduction of Curie temperature (Tbsubesub) with decreasing thickness, which is coherent with a mean field model description. The reduced ordering temperature also accounts for the thickness dependence of the magnetic anisotropy constants and resonance fields. The damping of the system is strongly thickness dependent, and is for thin films dominated by thickness dependent anisotropies, yielding both a strong two-magnon scattering close to Tbsubesub and a low temperature broadening. For the bulk like samples a large part of the broadening can be linked to spread in magnetic anisotropies attributed to crystal imperfections/domain boundaries of the bulk like film.

    Original languageEnglish (US)
    Pages (from-to)197-204
    Number of pages8
    JournalJournal of Magnetism and Magnetic Materials
    Volume369
    DOIs
    StatePublished - 2014

    Fingerprint

    Ferromagnetic resonance
    Pulsed lasers
    pulsed lasers
    Magnetic properties
    Magnetic anisotropy
    magnetic properties
    Magnetization
    cells
    Thin films
    ferromagnetic resonance
    SQUIDs
    Curie temperature
    Linewidth
    Temperature
    Anisotropy
    Damping
    Spectroscopy
    Scattering
    anisotropy
    Defects

    Keywords

    • Ferromagnetic resonance
    • Line-widths
    • LSMO
    • Thin film magnetism

    ASJC Scopus subject areas

    • Condensed Matter Physics
    • Electronic, Optical and Magnetic Materials

    Cite this

    Thickness dependence of dynamic and static magnetic properties of pulsed laser deposited La0.7Sr0.3MnO3 films on SrTiO3(001). / Monsen, Åsmund; Boschker, Jos E.; Macià, Ferran; Wells, Justin W.; Nordblad, Per; Kent, Andrew D.; Mathieu, Roland; Tybell, Thomas; Wahlström, Erik.

    In: Journal of Magnetism and Magnetic Materials, Vol. 369, 2014, p. 197-204.

    Research output: Contribution to journalArticle

    Monsen, Å, Boschker, JE, Macià, F, Wells, JW, Nordblad, P, Kent, AD, Mathieu, R, Tybell, T & Wahlström, E 2014, 'Thickness dependence of dynamic and static magnetic properties of pulsed laser deposited La0.7Sr0.3MnO3 films on SrTiO3(001)', Journal of Magnetism and Magnetic Materials, vol. 369, pp. 197-204. https://doi.org/10.1016/j.jmmm.2014.06.038
    Monsen, Åsmund ; Boschker, Jos E. ; Macià, Ferran ; Wells, Justin W. ; Nordblad, Per ; Kent, Andrew D. ; Mathieu, Roland ; Tybell, Thomas ; Wahlström, Erik. / Thickness dependence of dynamic and static magnetic properties of pulsed laser deposited La0.7Sr0.3MnO3 films on SrTiO3(001). In: Journal of Magnetism and Magnetic Materials. 2014 ; Vol. 369. pp. 197-204.
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    AU - Boschker, Jos E.

    AU - Macià, Ferran

    AU - Wells, Justin W.

    AU - Nordblad, Per

    AU - Kent, Andrew D.

    AU - Mathieu, Roland

    AU - Tybell, Thomas

    AU - Wahlström, Erik

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    N2 - We present a comprehensive study of the thickness dependence of static and magneto-dynamic magnetic properties of La0.7Sr0.3MnO 3. Epitaxial pulsed laser deposited La0.7Sr 0.3MnO3/SrTiO3(001) thin films in the range from 3 unit cell (uc) to 40 uc (1.2-16 nm) have been investigated through ferromagnetic resonance (FMR) spectroscopy and SQUID magnetometry at variable temperature. Magnetodynamically, three different thickness, d, regimes are identified: 20 uc ≲d uc where the system is bulk like, a transition region 8 uc ≤≲20 uc where the FMR linewidth and the position depend on thickness and d=6 uc which displays significantly altered magnetodynamic properties, while still displaying bulk magnetization. Magnetization and FMR measurements are consistent with a nonmagnetic volume corresponding to ∼4 uc. We observe a reduction of Curie temperature (Tbsubesub) with decreasing thickness, which is coherent with a mean field model description. The reduced ordering temperature also accounts for the thickness dependence of the magnetic anisotropy constants and resonance fields. The damping of the system is strongly thickness dependent, and is for thin films dominated by thickness dependent anisotropies, yielding both a strong two-magnon scattering close to Tbsubesub and a low temperature broadening. For the bulk like samples a large part of the broadening can be linked to spread in magnetic anisotropies attributed to crystal imperfections/domain boundaries of the bulk like film.

    AB - We present a comprehensive study of the thickness dependence of static and magneto-dynamic magnetic properties of La0.7Sr0.3MnO 3. Epitaxial pulsed laser deposited La0.7Sr 0.3MnO3/SrTiO3(001) thin films in the range from 3 unit cell (uc) to 40 uc (1.2-16 nm) have been investigated through ferromagnetic resonance (FMR) spectroscopy and SQUID magnetometry at variable temperature. Magnetodynamically, three different thickness, d, regimes are identified: 20 uc ≲d uc where the system is bulk like, a transition region 8 uc ≤≲20 uc where the FMR linewidth and the position depend on thickness and d=6 uc which displays significantly altered magnetodynamic properties, while still displaying bulk magnetization. Magnetization and FMR measurements are consistent with a nonmagnetic volume corresponding to ∼4 uc. We observe a reduction of Curie temperature (Tbsubesub) with decreasing thickness, which is coherent with a mean field model description. The reduced ordering temperature also accounts for the thickness dependence of the magnetic anisotropy constants and resonance fields. The damping of the system is strongly thickness dependent, and is for thin films dominated by thickness dependent anisotropies, yielding both a strong two-magnon scattering close to Tbsubesub and a low temperature broadening. For the bulk like samples a large part of the broadening can be linked to spread in magnetic anisotropies attributed to crystal imperfections/domain boundaries of the bulk like film.

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