### Abstract

We discuss the en tension of dynamic light scattering to very strongly scattering media, where the propagation of light is described by the diffusion approximation, allowing the distribution of the light paths to be determined. The temporal evolution of the length of each of these paths, due to the dynamics of the scattering medium, is calculated, and an expression for the temporal autocorrelation function of the intensity fluctuations of the scattered light is obtained. This relates the measured decay of the autocorrelation function to the dynamics of the medium. This technique is called diffusing wave spectroscopy (DWS). To extend its utility, we consider the consequences of interactions between the scattering particles on the light scattering. To illustrate its applications, we consider several examples of new physics that can be investigated using DWS. We study the transient nature of hydrodynamic interactions between a particle and the surrounding fluid. We are able to probe the decay of the velocity correlation function of the particles, and we demonstrate its algebraic decay, with a t^{-3/2}time dependence. We also show that the time-dependent self diffusion coefficient exhibits an unexpected scaling behavior, whereby all the data, from samples of different volume fractions, can be scaled onto a single curve. Finally, we discuss the applications of DWS to the study of the dynamics of foams, and show how it can be used to probe the rearrangement of the bubbles within the foam as they coarsen.

Original language | English (US) |
---|---|

Pages (from-to) | 610-621 |

Number of pages | 12 |

Journal | Physica Scripta |

Volume | 1993 |

Issue number | T49B |

DOIs | |

State | Published - Jan 1 1993 |

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### ASJC Scopus subject areas

- Condensed Matter Physics
- Mathematical Physics
- Atomic and Molecular Physics, and Optics

### Cite this

*Physica Scripta*,

*1993*(T49B), 610-621. https://doi.org/10.1088/0031-8949/1993/T49B/040

**Diffusing-wave spectroscopy : The technique and some applications.** / Weitz, D. A.; Gang, Hu; Pine, D. J.; Zhu, J. X.; Durian, D. J.

Research output: Contribution to journal › Article

*Physica Scripta*, vol. 1993, no. T49B, pp. 610-621. https://doi.org/10.1088/0031-8949/1993/T49B/040

}

TY - JOUR

T1 - Diffusing-wave spectroscopy

T2 - The technique and some applications

AU - Weitz, D. A.

AU - Gang, Hu

AU - Pine, D. J.

AU - Zhu, J. X.

AU - Durian, D. J.

PY - 1993/1/1

Y1 - 1993/1/1

N2 - We discuss the en tension of dynamic light scattering to very strongly scattering media, where the propagation of light is described by the diffusion approximation, allowing the distribution of the light paths to be determined. The temporal evolution of the length of each of these paths, due to the dynamics of the scattering medium, is calculated, and an expression for the temporal autocorrelation function of the intensity fluctuations of the scattered light is obtained. This relates the measured decay of the autocorrelation function to the dynamics of the medium. This technique is called diffusing wave spectroscopy (DWS). To extend its utility, we consider the consequences of interactions between the scattering particles on the light scattering. To illustrate its applications, we consider several examples of new physics that can be investigated using DWS. We study the transient nature of hydrodynamic interactions between a particle and the surrounding fluid. We are able to probe the decay of the velocity correlation function of the particles, and we demonstrate its algebraic decay, with a t-3/2time dependence. We also show that the time-dependent self diffusion coefficient exhibits an unexpected scaling behavior, whereby all the data, from samples of different volume fractions, can be scaled onto a single curve. Finally, we discuss the applications of DWS to the study of the dynamics of foams, and show how it can be used to probe the rearrangement of the bubbles within the foam as they coarsen.

AB - We discuss the en tension of dynamic light scattering to very strongly scattering media, where the propagation of light is described by the diffusion approximation, allowing the distribution of the light paths to be determined. The temporal evolution of the length of each of these paths, due to the dynamics of the scattering medium, is calculated, and an expression for the temporal autocorrelation function of the intensity fluctuations of the scattered light is obtained. This relates the measured decay of the autocorrelation function to the dynamics of the medium. This technique is called diffusing wave spectroscopy (DWS). To extend its utility, we consider the consequences of interactions between the scattering particles on the light scattering. To illustrate its applications, we consider several examples of new physics that can be investigated using DWS. We study the transient nature of hydrodynamic interactions between a particle and the surrounding fluid. We are able to probe the decay of the velocity correlation function of the particles, and we demonstrate its algebraic decay, with a t-3/2time dependence. We also show that the time-dependent self diffusion coefficient exhibits an unexpected scaling behavior, whereby all the data, from samples of different volume fractions, can be scaled onto a single curve. Finally, we discuss the applications of DWS to the study of the dynamics of foams, and show how it can be used to probe the rearrangement of the bubbles within the foam as they coarsen.

UR - http://www.scopus.com/inward/record.url?scp=84956075218&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=84956075218&partnerID=8YFLogxK

U2 - 10.1088/0031-8949/1993/T49B/040

DO - 10.1088/0031-8949/1993/T49B/040

M3 - Article

VL - 1993

SP - 610

EP - 621

JO - Physica Scripta

JF - Physica Scripta

SN - 0031-8949

IS - T49B

ER -