Characterizing equilibrium in epitaxial growth

P. N. Patrone, Russel Caflisch, D. Margetis

Research output: Contribution to journalArticle

Abstract

Using a kinetic model of epitaxial growth, we describe how geometry controls kinetic pathways through which external deposition influences the state of a vicinal surface. The state of the surface is determined by three key, adjustable parameters: the local step angle θ, the Péclet number P, and the single-bond detachment rate . By scaling arguments in P, we find three steady-state regimes. In one regime, detailed flux balance approximately holds, so that the system is near equilibrium. In the other two regimes, geometric effects compete with deposition as the system is driven progressively out of equilibrium. Our analytical results are in excellent agreement with those of kinetic Monte Carlo simulations.

Original languageEnglish (US)
Article number48012
JournalEPL
Volume97
Issue number4
DOIs
StatePublished - Feb 2012

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kinetics
detachment
scaling
geometry
simulation

ASJC Scopus subject areas

  • Physics and Astronomy(all)

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Patrone, P. N., Caflisch, R., & Margetis, D. (2012). Characterizing equilibrium in epitaxial growth. EPL, 97(4), [48012]. https://doi.org/10.1209/0295-5075/97/48012

Characterizing equilibrium in epitaxial growth. / Patrone, P. N.; Caflisch, Russel; Margetis, D.

In: EPL, Vol. 97, No. 4, 48012, 02.2012.

Research output: Contribution to journalArticle

Patrone, PN, Caflisch, R & Margetis, D 2012, 'Characterizing equilibrium in epitaxial growth', EPL, vol. 97, no. 4, 48012. https://doi.org/10.1209/0295-5075/97/48012
Patrone PN, Caflisch R, Margetis D. Characterizing equilibrium in epitaxial growth. EPL. 2012 Feb;97(4). 48012. https://doi.org/10.1209/0295-5075/97/48012
Patrone, P. N. ; Caflisch, Russel ; Margetis, D. / Characterizing equilibrium in epitaxial growth. In: EPL. 2012 ; Vol. 97, No. 4.
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